Deposition and Evaporation of Polychlorobiphenyl Congeners to and from Siskiwit Lake, Isle Royale, Lake Superior

Swackhamer DL, Mcveety BD, Hites RA. 1988. Deposition and Evaporation of Polychlorobiphenyl Congeners to and from Siskiwit Lake, Isle Royale, Lake Superior. Environmental Science & Technology. 22(6):664-672

The relative importance of polychlorobiphenyl (PCB) transport into and out of lakes was studied by constructing a mass balance of PCB congeners in Siskiwit Lake, a remote lake in Isle Royale National Park in Lake Superior. Measurements of winter and summer air, rain, snow, water, and sediments were obtained over several months and used to determine PCB flluxes to and from the lake, assuming steady-state conditions over 1 year. By solving the mass balance equation under selected conditions, the deposition velocity and the overall liquid water-to-air mass transfer coefficient for PCBs was estimated. Wet depositionwas generally 3 times as gret as dry deposition and was dominated by particle washout. Rain was a more important removal process than snow. Removal from the lake by volatization was more important than sedimentation for most congeners.

Type
Journal Article
Authors
Swackhamer, Deborah; Mcveety, Bruce; Hites, Ronald
Units
ISRO
Keywords
Aquatic Sciences, Atmospheric Sciences, PCB

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